A roadmap for electronic grade 2D materials

Natalie Briggs, Shruti Subramanian, Zhong Lin, Xufan Li, Xiaotian Zhang, Kehao Zhang, Kai Xiao, David Geohegan, Robert Wallace, Long Qing Chen, Mauricio Terrones, Aida Ebrahimi, Saptarshi Das, Joan Redwing, Christopher Hinkle, Kasra Momeni, Adri Van Duin, Vin Crespi, Swastik Kar, Joshua A. Robinson

Research output: Contribution to journalReview article

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Abstract

Since their modern debut in 2004, 2-dimensional (2D) materials continue to exhibit scientific and industrial promise, providing a broad materials platform for scientific investigation, and development of nano- A nd atomic-scale devices. A significant focus of the last decade's research in this field has been 2D semiconductors, whose electronic properties can be tuned through manipulation of dimensionality, substrate engineering, strain, and doping (Mak et al 2010 Phys. Rev. Lett. 105 136805; Zhang et al 2017 Sci. Rep. 7 16938; Conley et al 2013 Nano Lett. 13 3626-30; Li et al 2016 Adv. Mater. 28 8240-7; Rhodes et al 2017 Nano Lett. 17 1616-22; Gong et al 2014 Nano Lett. 14 442-9; Suh et al 2014 Nano Lett. 14 6976-82; Yoshida et al 2015 Sci. Rep. 5 14808). Molybdenum disulfide (MoS2) and tungsten diselenide (WSe2) have dominated recent interest for potential integration in electronic technologies, due to their intrinsic and tunable properties, atomic-scale thicknesses, and relative ease of stacking to create new and custom structures. However, to go 'beyond the bench', advances in large-scale, 2D layer synthesis and engineering must lead to 'exfoliation-quality' 2D layers at the wafer scale. This roadmap aims to address this grand challenge by identifying key technology drivers where 2D layers can have an impact, and to discuss synthesis and layer engineering for the realization of electronic-grade, 2D materials. We focus on three fundamental areas of research that must be heavily pursued in both experiment and computation to achieve high-quality materials for electronic and optoelectronic applications.

Original languageEnglish (US)
Article number022001
Journal2D Materials
Volume6
Issue number2
DOIs
StatePublished - Jan 17 2019

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All Science Journal Classification (ASJC) codes

  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering

Cite this

Briggs, N., Subramanian, S., Lin, Z., Li, X., Zhang, X., Zhang, K., Xiao, K., Geohegan, D., Wallace, R., Chen, L. Q., Terrones, M., Ebrahimi, A., Das, S., Redwing, J., Hinkle, C., Momeni, K., Van Duin, A., Crespi, V., Kar, S., & Robinson, J. A. (2019). A roadmap for electronic grade 2D materials. 2D Materials, 6(2), [022001]. https://doi.org/10.1088/2053-1583/aaf836