Bismuth Telluride/Half-Heusler Segmented Thermoelectric Unicouple Modules Provide 12% Conversion Efficiency

Wenjie Li, Bed Poudel, Amin Nozariasbmarz, Rammohan Sriramdas, Hangtian Zhu, Han Byul Kang, Shashank Priya

Research output: Contribution to journalArticlepeer-review

1 Scopus citations

Abstract

The rapid enhancement of the thermoelectric (TE) figure-of-merit (zT) in the past decade has opened opportunities for developing and transitioning solid state waste heat recovery systems. Here, a segmented TE device architecture is demonstrated in conjunction with heterogeneous material integration that results in high unicouple-level conversion efficiency of 12% under a temperature difference of 584 K. This breakthrough is the result of success in fabricating bismuth telluride/half-Heusler segmented TE unicouple modules using a “hot-to-cold” fabrication technique that provides significantly reduced electrical and thermal contact resistance. Extensive analytical and finite element modeling is conducted to provide an understanding of the nature of thermal transport and contributions arising from various thermal and physical parameters. Bismuth telluride/half-Heusler based segmented thermoelectric generators (TEGs) can provide higher practical temperature difference with optimum average zT across the whole operating range. These results will have immediate impact on the design and development of TEGs and in the general design of devices based upon heterostructures that take advantage of gradients in the figure of merit.

Original languageEnglish (US)
Article number2001924
JournalAdvanced Energy Materials
Volume10
Issue number38
DOIs
StatePublished - Oct 1 2020

All Science Journal Classification (ASJC) codes

  • Renewable Energy, Sustainability and the Environment
  • Materials Science(all)

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