Coal seam porosity and fracture heterogeneity of macrolithotypes in the Hancheng Block, eastern margin, Ordos Basin, China

Junlong Zhao, Hao Xu, Dazhen Tang, Jonathan P. Mathews, Song Li, Shu Tao

Research output: Contribution to journalArticle

44 Citations (Scopus)

Abstract

Heterogeneity in cleats and pore size distribution within coal macrolithotypes (bright, semi-bright, semi-dull, and dull coals, determined from the overall relative luster and percentage of bright components) impact coalbed methane (CBM) extraction. However, few studies have investigated the characteristics of macrolithotypes across multiple length scales. Here, the macrolithotype description was performed for the No. 3, 5, and 11 coal seams in the Hancheng Block of Ordos Basin. The cleats were characterized by optical microscopy and X-ray computed tomography (CT) while pores and their connectivity were determined from mercury intrusion porosimetry, N2 and CO2 adsorption, and low field nuclear magnetic resonance (NMR) of water saturated cores evaluated both cleats and pores. The CH4 adsorption capacity of coal samples scraped from the surface of the macrolithotype layers was also determined. Dull lithotypes (semi-dull and dull) were dominant, followed by bright lithotypes (bright and semi-bright) in these seams. The bright lithotype coal has a higher microfracture density (averaging 339 microcleats per 9 cm2, μm-mm), better connectivity, and a larger fractal dimension (averaging 1.7) from optical microscopy. The dull lithotype has a lower average microfracture density (272 microcleats per 9 cm2) and a smaller fractal dimension (~1.6). This higher connectivity observation was consistent with X-ray CT observations and low field NMR of the water saturated cores (and the transition upon water removal from the fractures and larger pores). Also the ease of mercury injection from cores also supported higher connectivity in the bright lithotypes. Both the semi-bright and semi-dull lithotypes have equivalent pore proportions micro- to macropores and good apparent connectivity at the nm-μm scale; despite mineral occlusions. Based on the CH4 adsorption capacities of the macrolithotypes, the bright coal has the greatest gas adsorption capacity, due to the largest smaller micropores (<2 nm) and a higher specific surface area. These observations aid in understanding the complex behavior observed in CBM extraction and evaluating the impacts of heterogeneity and scale on the degassing behavior.

Original languageEnglish (US)
Pages (from-to)18-29
Number of pages12
JournalInternational Journal of Coal Geology
Volume159
DOIs
StatePublished - Apr 1 2016

Fingerprint

lithotype
coal seam
Porosity
porosity
Coal
connectivity
coal
basin
adsorption
coalbed methane
Fractal dimension
Adsorption
tomography
Optical microscopy
Tomography
nuclear magnetic resonance
microscopy
Nuclear magnetic resonance
Water
X rays

All Science Journal Classification (ASJC) codes

  • Fuel Technology
  • Geology
  • Economic Geology
  • Stratigraphy

Cite this

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title = "Coal seam porosity and fracture heterogeneity of macrolithotypes in the Hancheng Block, eastern margin, Ordos Basin, China",
abstract = "Heterogeneity in cleats and pore size distribution within coal macrolithotypes (bright, semi-bright, semi-dull, and dull coals, determined from the overall relative luster and percentage of bright components) impact coalbed methane (CBM) extraction. However, few studies have investigated the characteristics of macrolithotypes across multiple length scales. Here, the macrolithotype description was performed for the No. 3, 5, and 11 coal seams in the Hancheng Block of Ordos Basin. The cleats were characterized by optical microscopy and X-ray computed tomography (CT) while pores and their connectivity were determined from mercury intrusion porosimetry, N2 and CO2 adsorption, and low field nuclear magnetic resonance (NMR) of water saturated cores evaluated both cleats and pores. The CH4 adsorption capacity of coal samples scraped from the surface of the macrolithotype layers was also determined. Dull lithotypes (semi-dull and dull) were dominant, followed by bright lithotypes (bright and semi-bright) in these seams. The bright lithotype coal has a higher microfracture density (averaging 339 microcleats per 9 cm2, μm-mm), better connectivity, and a larger fractal dimension (averaging 1.7) from optical microscopy. The dull lithotype has a lower average microfracture density (272 microcleats per 9 cm2) and a smaller fractal dimension (~1.6). This higher connectivity observation was consistent with X-ray CT observations and low field NMR of the water saturated cores (and the transition upon water removal from the fractures and larger pores). Also the ease of mercury injection from cores also supported higher connectivity in the bright lithotypes. Both the semi-bright and semi-dull lithotypes have equivalent pore proportions micro- to macropores and good apparent connectivity at the nm-μm scale; despite mineral occlusions. Based on the CH4 adsorption capacities of the macrolithotypes, the bright coal has the greatest gas adsorption capacity, due to the largest smaller micropores (<2 nm) and a higher specific surface area. These observations aid in understanding the complex behavior observed in CBM extraction and evaluating the impacts of heterogeneity and scale on the degassing behavior.",
author = "Junlong Zhao and Hao Xu and Dazhen Tang and Mathews, {Jonathan P.} and Song Li and Shu Tao",
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Coal seam porosity and fracture heterogeneity of macrolithotypes in the Hancheng Block, eastern margin, Ordos Basin, China. / Zhao, Junlong; Xu, Hao; Tang, Dazhen; Mathews, Jonathan P.; Li, Song; Tao, Shu.

In: International Journal of Coal Geology, Vol. 159, 01.04.2016, p. 18-29.

Research output: Contribution to journalArticle

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N2 - Heterogeneity in cleats and pore size distribution within coal macrolithotypes (bright, semi-bright, semi-dull, and dull coals, determined from the overall relative luster and percentage of bright components) impact coalbed methane (CBM) extraction. However, few studies have investigated the characteristics of macrolithotypes across multiple length scales. Here, the macrolithotype description was performed for the No. 3, 5, and 11 coal seams in the Hancheng Block of Ordos Basin. The cleats were characterized by optical microscopy and X-ray computed tomography (CT) while pores and their connectivity were determined from mercury intrusion porosimetry, N2 and CO2 adsorption, and low field nuclear magnetic resonance (NMR) of water saturated cores evaluated both cleats and pores. The CH4 adsorption capacity of coal samples scraped from the surface of the macrolithotype layers was also determined. Dull lithotypes (semi-dull and dull) were dominant, followed by bright lithotypes (bright and semi-bright) in these seams. The bright lithotype coal has a higher microfracture density (averaging 339 microcleats per 9 cm2, μm-mm), better connectivity, and a larger fractal dimension (averaging 1.7) from optical microscopy. The dull lithotype has a lower average microfracture density (272 microcleats per 9 cm2) and a smaller fractal dimension (~1.6). This higher connectivity observation was consistent with X-ray CT observations and low field NMR of the water saturated cores (and the transition upon water removal from the fractures and larger pores). Also the ease of mercury injection from cores also supported higher connectivity in the bright lithotypes. Both the semi-bright and semi-dull lithotypes have equivalent pore proportions micro- to macropores and good apparent connectivity at the nm-μm scale; despite mineral occlusions. Based on the CH4 adsorption capacities of the macrolithotypes, the bright coal has the greatest gas adsorption capacity, due to the largest smaller micropores (<2 nm) and a higher specific surface area. These observations aid in understanding the complex behavior observed in CBM extraction and evaluating the impacts of heterogeneity and scale on the degassing behavior.

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