Combined carbon mesh and small graphite fiber brush anodes to enhance and stabilize power generation in microbial fuel cells treating domestic wastewater

Shijia Wu, Weihua He, Wulin Yang, Yaoli Ye, Xia Huang, Bruce Ernest Logan

Research output: Contribution to journalArticle

31 Citations (Scopus)

Abstract

Microbial fuel cells (MFCs) need to have a compact architecture, but power generation using low strength domestic wastewater is unstable for closely-spaced electrode designs using thin anodes (flat mesh or small diameter graphite fiber brushes) due to oxygen crossover from the cathode. A composite anode configuration was developed to improve performance, by joining the mesh and brushes together, with the mesh used to block oxygen crossover to the brushes, and the brushes used to stabilize mesh potentials. In small, fed-batch MFCs (28 mL), the composite anode produced 20% higher power densities than MFCs using only brushes, and 150% power densities compared to carbon mesh anodes. In continuous flow tests at short hydraulic retention times (HRTs, 2 or 4 h) using larger MFCs (100 mL), composite anodes had stable performance, while brush anode MFCs exhibited power overshoot in polarization tests. Both configurations exhibited power overshoot at a longer HRT of 8 h due to lower effluent CODs. The use of composite anodes reduced biomass growth on the cathode (1.9 ± 0.2 mg) compared to only brushes (3.1 ± 0.3 mg), and increased coulombic efficiencies, demonstrating that they successfully reduced oxygen contamination of the anode and the bio-fouling of cathode.

Original languageEnglish (US)
Pages (from-to)348-355
Number of pages8
JournalJournal of Power Sources
Volume356
DOIs
StatePublished - Jan 1 2017

Fingerprint

Graphite fibers
Microbial fuel cells
brushes
Brushes
fuel cells
Power generation
mesh
Anodes
Wastewater
anodes
Carbon
graphite
fibers
carbon
Cathodes
composite materials
cathodes
Composite materials
Oxygen
radiant flux density

All Science Journal Classification (ASJC) codes

  • Renewable Energy, Sustainability and the Environment
  • Energy Engineering and Power Technology
  • Physical and Theoretical Chemistry
  • Electrical and Electronic Engineering

Cite this

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title = "Combined carbon mesh and small graphite fiber brush anodes to enhance and stabilize power generation in microbial fuel cells treating domestic wastewater",
abstract = "Microbial fuel cells (MFCs) need to have a compact architecture, but power generation using low strength domestic wastewater is unstable for closely-spaced electrode designs using thin anodes (flat mesh or small diameter graphite fiber brushes) due to oxygen crossover from the cathode. A composite anode configuration was developed to improve performance, by joining the mesh and brushes together, with the mesh used to block oxygen crossover to the brushes, and the brushes used to stabilize mesh potentials. In small, fed-batch MFCs (28 mL), the composite anode produced 20{\%} higher power densities than MFCs using only brushes, and 150{\%} power densities compared to carbon mesh anodes. In continuous flow tests at short hydraulic retention times (HRTs, 2 or 4 h) using larger MFCs (100 mL), composite anodes had stable performance, while brush anode MFCs exhibited power overshoot in polarization tests. Both configurations exhibited power overshoot at a longer HRT of 8 h due to lower effluent CODs. The use of composite anodes reduced biomass growth on the cathode (1.9 ± 0.2 mg) compared to only brushes (3.1 ± 0.3 mg), and increased coulombic efficiencies, demonstrating that they successfully reduced oxygen contamination of the anode and the bio-fouling of cathode.",
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Combined carbon mesh and small graphite fiber brush anodes to enhance and stabilize power generation in microbial fuel cells treating domestic wastewater. / Wu, Shijia; He, Weihua; Yang, Wulin; Ye, Yaoli; Huang, Xia; Logan, Bruce Ernest.

In: Journal of Power Sources, Vol. 356, 01.01.2017, p. 348-355.

Research output: Contribution to journalArticle

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AU - Logan, Bruce Ernest

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