Denuder measurements of gas and aerosol species above Arctic snow surfaces at Alert 2000

Antonietta Ianniello, Harald J. Beine, Roberto Sparapani, Francesca Di Bari, Ivo Allegrini, Jose Fuentes

Research output: Contribution to journalArticlepeer-review

23 Scopus citations

Abstract

Gas and aerosol measurements were made during the Polar Sunrise Experiment 2000 at Alert, Nunavut (Canada), using two independent denuder/filter systems for sampling and subsequent analysis by ion chromatography. Twelve to forty-eight hour samples were taken during a winter (9-21 February 2000) and a spring (17 April-5 May 2000) campaign. During the spring campaign, samples were taken at two different heights above the snow surface to investigate concentration differences. Total particulate NO3- is the most abundant inorganic nitrogen compound during Arctic springtime (mean 137.4ngm-3). The NO3- fluxes were calculated above the snow surface to help identify processes that control snow-atmosphere exchange of reactive nitrogen compounds. We suggest that the observed fluxes of coarse particle NO3- via snow deposition may contribute to the nitrogen inventory in the snow surface. Measurements of surface snow provide experimental data that constrain the contribution of dry deposition of coarse particle NO3- to <7%. Wet deposition in falling snow appears to be the major contributor to the nitrate input to the snow.

Original languageEnglish (US)
Pages (from-to)5299-5309
Number of pages11
JournalAtmospheric Environment
Volume36
Issue number34
DOIs
StatePublished - Nov 1 2002

All Science Journal Classification (ASJC) codes

  • Environmental Science(all)
  • Atmospheric Science

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