Abstract
The abundance distribution of neutral Cun clusters sputtered by 5 keV Ar impact from a polycrystalline Cu surface is measured using single-photon laser post-ionization. Molecular dynamics computer simulation is used to gain insight into the cluster sputtering process. Three different codes and two potentials are used to check the sensitivity of the results on numerics and physical input. Differences in the results obtained by the various codes and the different potentials used are discussed. While the total sputter yield is consistent with experiment, the fraction of atoms bound in clusters, and in particular the dimer fraction, are overestimated by at least a factor of 4. This is also true for a many-body potential which has been fitted to describe both bulk Cu and dimers. In detail, the simulation shows that larger clusters are emitted at later times from the target. Clusters originate mainly from regions of the surface, which are around the melting temperature of bulk Cu. Large clusters are emitted preferably from ion impacts with a high individual sputter yield. Finally, we simulate sputtering from a model Cu material with an artificially decreased cohesive energy. Here, drastic high-yield events (up to Y = 78) can be observed, which produce clusters abundantly.
| Original language | English (US) |
|---|---|
| Pages (from-to) | 284-297 |
| Number of pages | 14 |
| Journal | Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms |
| Volume | 143 |
| Issue number | 3 |
| DOIs | |
| State | Published - Sep 1 1998 |
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All Science Journal Classification (ASJC) codes
- Nuclear and High Energy Physics
- Instrumentation
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Experiment and simulation of cluster emission from 5 keV Ar → Cu. / Colla, Th J.; Urbassek, H. M.; Wucher, A.; Staudt, C.; Heinrich, R.; Garrison, Barbara Jane; Dandachi, C.; Betz, G.
In: Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms, Vol. 143, No. 3, 01.09.1998, p. 284-297.Research output: Contribution to journal › Article
TY - JOUR
T1 - Experiment and simulation of cluster emission from 5 keV Ar → Cu
AU - Colla, Th J.
AU - Urbassek, H. M.
AU - Wucher, A.
AU - Staudt, C.
AU - Heinrich, R.
AU - Garrison, Barbara Jane
AU - Dandachi, C.
AU - Betz, G.
PY - 1998/9/1
Y1 - 1998/9/1
N2 - The abundance distribution of neutral Cun clusters sputtered by 5 keV Ar impact from a polycrystalline Cu surface is measured using single-photon laser post-ionization. Molecular dynamics computer simulation is used to gain insight into the cluster sputtering process. Three different codes and two potentials are used to check the sensitivity of the results on numerics and physical input. Differences in the results obtained by the various codes and the different potentials used are discussed. While the total sputter yield is consistent with experiment, the fraction of atoms bound in clusters, and in particular the dimer fraction, are overestimated by at least a factor of 4. This is also true for a many-body potential which has been fitted to describe both bulk Cu and dimers. In detail, the simulation shows that larger clusters are emitted at later times from the target. Clusters originate mainly from regions of the surface, which are around the melting temperature of bulk Cu. Large clusters are emitted preferably from ion impacts with a high individual sputter yield. Finally, we simulate sputtering from a model Cu material with an artificially decreased cohesive energy. Here, drastic high-yield events (up to Y = 78) can be observed, which produce clusters abundantly.
AB - The abundance distribution of neutral Cun clusters sputtered by 5 keV Ar impact from a polycrystalline Cu surface is measured using single-photon laser post-ionization. Molecular dynamics computer simulation is used to gain insight into the cluster sputtering process. Three different codes and two potentials are used to check the sensitivity of the results on numerics and physical input. Differences in the results obtained by the various codes and the different potentials used are discussed. While the total sputter yield is consistent with experiment, the fraction of atoms bound in clusters, and in particular the dimer fraction, are overestimated by at least a factor of 4. This is also true for a many-body potential which has been fitted to describe both bulk Cu and dimers. In detail, the simulation shows that larger clusters are emitted at later times from the target. Clusters originate mainly from regions of the surface, which are around the melting temperature of bulk Cu. Large clusters are emitted preferably from ion impacts with a high individual sputter yield. Finally, we simulate sputtering from a model Cu material with an artificially decreased cohesive energy. Here, drastic high-yield events (up to Y = 78) can be observed, which produce clusters abundantly.
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U2 - 10.1016/S0168-583X(98)00336-X
DO - 10.1016/S0168-583X(98)00336-X
M3 - Article
AN - SCOPUS:0032162789
VL - 143
SP - 284
EP - 297
JO - Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms
JF - Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms
SN - 0168-583X
IS - 3
ER -