From (π,0) magnetic order to superconductivity with (π,π) magnetic resonance in Fe1.02 Te1-x Sex

T. J. Liu, J. Hu, B. Qian, D. Fobes, Z. Q. Mao, W. Bao, M. Reehuis, S. A.J. Kimber, K. ProkeŠ, S. Matas, D. N. Argyriou, A. Hiess, A. Rotaru, H. Pham, L. Spinu, Y. Qiu, V. Thampy, A. T. Savici, J. A. Rodriguez, C. Broholm

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Abstract

The iron chalcogenide Fe 1+y (Te 1-x Se x) is structurally the simplest of the Fe-based superconductors. Although the Fermi surface is similar to iron pnictides, the parent compoundFe 1+y Te exhibits antiferromagnetic order with an in-plane magnetic wave vector (π,0) (ref. 6). This contrasts the pnictide parent compounds where the magnetic order has an in-plane magnetic wave vector (π,π) that connects hole and electron parts of the Fermi surface. Despite these differences, both the pnictide and chalcogenide Fe superconductors exhibit a superconducting spin resonance around (π,π) (ref. 9, 10, 11). A central question in this burgeoning field is therefore how (π,π) superconductivity can emerge from a (π,0) magnetic instability. Here, we report that the magnetic soft mode evolving from the (π,0)-type magnetic long-range order is associated with weak charge carrier localization. Bulk superconductivity occurs as magnetic correlations at (π,0) are suppressed and the mode at (π, π) becomes dominant for x>0.29. Our results suggest a common magnetic origin for superconductivity in iron chalcogenide and pnictide superconductors.

Original languageEnglish (US)
Pages (from-to)716-720
Number of pages5
JournalNature Materials
Volume9
Issue number9
DOIs
StatePublished - Sep 2010

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All Science Journal Classification (ASJC) codes

  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering

Cite this

Liu, T. J., Hu, J., Qian, B., Fobes, D., Mao, Z. Q., Bao, W., Reehuis, M., Kimber, S. A. J., ProkeŠ, K., Matas, S., Argyriou, D. N., Hiess, A., Rotaru, A., Pham, H., Spinu, L., Qiu, Y., Thampy, V., Savici, A. T., Rodriguez, J. A., & Broholm, C. (2010). From (π,0) magnetic order to superconductivity with (π,π) magnetic resonance in Fe1.02 Te1-x Sex. Nature Materials, 9(9), 716-720. https://doi.org/10.1038/nmat2800