TY - JOUR
T1 - Graphene and Beyond
T2 - Recent Advances in Two-Dimensional Materials Synthesis, Properties, and Devices
AU - Lei, Yu
AU - Zhang, Tianyi
AU - Lin, Yu Chuan
AU - Granzier-Nakajima, Tomotaroh
AU - Bepete, George
AU - Kowalczyk, Dorota A.
AU - Lin, Zhong
AU - Zhou, Da
AU - Schranghamer, Thomas F.
AU - Dodda, Akhil
AU - Sebastian, Amritanand
AU - Chen, Yifeng
AU - Liu, Yuanyue
AU - Pourtois, Geoffrey
AU - Kempa, Thomas J.
AU - Schuler, Bruno
AU - Edmonds, Mark T.
AU - Quek, Su Ying
AU - Wurstbauer, Ursula
AU - Wu, Stephen M.
AU - Glavin, Nicholas R.
AU - Das, Saptarshi
AU - Dash, Saroj Prasad
AU - Redwing, Joan M.
AU - Robinson, Joshua A.
AU - Terrones, Mauricio
N1 - Funding Information:
J.A.R., G.B., Y.L., and M.T. thank the National Science Foundation- I/UCRC Phase II the Pennsylvania State University: Center for Atomically Thin Multifunctional Coatings (ATOMIC); grant No. 2113864 for partial support. This work was also partially supported by an Air Force Office of Scientific Research Grants: FA9550-18-1-0072 and FA9550-18-1-0283. Y.L. would like to acknowledge the Scientific Research Start-up Funds (No. QD2021033C) at Tsinghua Shenzhen International Graduate School. Y.-C.L. and J.A.R. acknowledge funding from NEWLIMITS, a center in nCORE as part of the Semiconductor Research Corporation (SRC) program sponsored by NIST through award number 70NANB17H041. J.A.R. and M.T. thank The Center for Nanoscale Science, a Materials Research Science and Engineering Center (MRSEC) supported by the National Science Foundation under grant DMR-2011839. M.T.E. acknowledges funding support from the Australian Research Council Discovery Project DP200101345 and M.T.E. was supported by Australian Research Council DECRA fellowship DE160101157. S.Y.Q. and Y.C. acknowledge funding from the Ministry of Education in Singapore under MOE2018-T3-1-005, and support from the Singapore National Research Foundation, Prime Minister’s Office, under its medium-sized center program. S.M.W. acknowledges support from the National Science Foundation (OMA-1936250 and ECCS-1942815). B.S. appreciates funding from the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation program (Grant agreement No. 948243). S.P.D. acknowledges European Union Graphene Flagship (Core 3, No. 881603), Sweden 2D TECH VINNOVA competence center at Chalmers University of Technology (No. 2019-00068). U.W. gratefully acknowledges financial support by the Deutsche Forschungsgemeinschaft (DFG) via Projects No. WU 637/4-2 No. WU 637/7-1 and the excellence cluster e-conversion–EXC 2089/1-390776260. D.A.K acknowledges the financial support from the National Science Centre, Poland (2016/21/B/ST5/00984, 2018/30/E/ST5/00667). Y. Liu acknowledges the support by Welch Foundation (F-1959-20210327), National Science Foundation (1900039), and ACS PRF (60934-DNI6). G.P. thanks imec and its IIAP core partner program for funding. G.P. is also grateful to Esteban A. Marques, Ashish Dabral, Benjamin Groven, Michiel J. van Setten, Sergiu Clima, Kiroubanand Sankaran, B. van Troeye, Daire Cott, P. Morin, V. Voronenkov, Aryan Afzalian, Sven Van Elshocht, Michel Houssa, Cedric Huyghebaert, and Iuliana Radu for their technical support. N.G. acknowledges support from the Asian Office of Aerospace Research and Development within the Air Force Office of Scientific Research grant #21IOA110 and support from the Air Force Office of Scientific Research under grant number 20RXCOR057. T.J.K. acknowledges funding by the Young Faculty Award program of the Defense Advanced Research Projects Agency (DARPA) and by the Army Research Office under the grant W911NF-21-1-0351. The views, opinions, and/or findings expressed are those of the authors and should not be interpreted as representing the official views or policies of the Department of Defense or the U.S. Government. T.J.K. also acknowledges funding from a National Science Foundation (DMR-1848046) CAREER grant. J.M.R. and J.A.R. acknowledge financial support from the 2D Crystal Consortium–Materials Innovation Platform (2DCC-MIP) facility at the Pennsylvania State University which is funded by the National Science Foundation under cooperative agreement DMR-2039351.
Publisher Copyright:
© 2022 American Chemical Society.
PY - 2022/12/21
Y1 - 2022/12/21
N2 - Since the isolation of graphene in 2004, two-dimensional (2D) materials research has rapidly evolved into an entire subdiscipline in the physical sciences with a wide range of emergent applications. The unique 2D structure offers an open canvas to tailor and functionalize 2D materials through layer number, defects, morphology, moiré pattern, strain, and other control knobs. Through this review, we aim to highlight the most recent discoveries in the following topics: theory-guided synthesis for enhanced control of 2D morphologies, quality, yield, as well as insights toward novel 2D materials; defect engineering to control and understand the role of various defects, including in situ and ex situ methods; and properties and applications that are related to moiré engineering, strain engineering, and artificial intelligence. Finally, we also provide our perspective on the challenges and opportunities in this fascinating field.
AB - Since the isolation of graphene in 2004, two-dimensional (2D) materials research has rapidly evolved into an entire subdiscipline in the physical sciences with a wide range of emergent applications. The unique 2D structure offers an open canvas to tailor and functionalize 2D materials through layer number, defects, morphology, moiré pattern, strain, and other control knobs. Through this review, we aim to highlight the most recent discoveries in the following topics: theory-guided synthesis for enhanced control of 2D morphologies, quality, yield, as well as insights toward novel 2D materials; defect engineering to control and understand the role of various defects, including in situ and ex situ methods; and properties and applications that are related to moiré engineering, strain engineering, and artificial intelligence. Finally, we also provide our perspective on the challenges and opportunities in this fascinating field.
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U2 - 10.1021/acsnanoscienceau.2c00017
DO - 10.1021/acsnanoscienceau.2c00017
M3 - Review article
C2 - 36573124
AN - SCOPUS:85139295630
SN - 2694-2496
VL - 2
SP - 450
EP - 485
JO - ACS Nanoscience Au
JF - ACS Nanoscience Au
IS - 6
ER -