High-energy storage performance of (Pb0.87Ba0.1la0.02)(Zr0.68Sn0.24Ti0.08)O3 antiferroelectric ceramics fabricated by the hot-press sintering method

Guangzu Zhang, Dingyang Zhu, Xiaoshan Zhang, Ling Zhang, Jinqiao Yi, Bing Xie, Yike Zeng, Qi Li, Qing Wang, Shenglin Jiang

Research output: Contribution to journalArticle

88 Citations (Scopus)

Abstract

(Pb0.87Ba0.1La0.02)(Zr0.68Sn0.24Ti0.08)O3 (PBLZST) antiferroelectric (AFE) ceramics have been prepared by hot-press sintering method and conventional solid-state reaction process, and the dependence of microstructure and energy storage properties of the ceramics on sintering approaches has been studied. The results reveal that not only the microstructure, but also the electrical properties of the PBLZST AFE ceramics are significantly improved by using the hot-press sintering method. Samples resulting from the hot-press sintering process have high breakdown strength of 180 kV/cm which results from the increase of density. Coupled with large polarization, the hotpressed AFE ceramics are shown to have a high recoverable energy density of 3.2 J/cm3. The recoverable energy density of the hot-pressed PBLZST AFE ceramics is 100% greater than the conventional sintered specimens with recoverable energy density of 1.6 J/cm3.

Original languageEnglish (US)
Pages (from-to)1175-1181
Number of pages7
JournalJournal of the American Ceramic Society
Volume98
Issue number4
DOIs
StatePublished - Jan 1 2015

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Energy storage
Sintering
Microstructure
Solid state reactions
Electric properties
Polarization

All Science Journal Classification (ASJC) codes

  • Ceramics and Composites
  • Materials Chemistry

Cite this

Zhang, Guangzu ; Zhu, Dingyang ; Zhang, Xiaoshan ; Zhang, Ling ; Yi, Jinqiao ; Xie, Bing ; Zeng, Yike ; Li, Qi ; Wang, Qing ; Jiang, Shenglin. / High-energy storage performance of (Pb0.87Ba0.1la0.02)(Zr0.68Sn0.24Ti0.08)O3 antiferroelectric ceramics fabricated by the hot-press sintering method. In: Journal of the American Ceramic Society. 2015 ; Vol. 98, No. 4. pp. 1175-1181.
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abstract = "(Pb0.87Ba0.1La0.02)(Zr0.68Sn0.24Ti0.08)O3 (PBLZST) antiferroelectric (AFE) ceramics have been prepared by hot-press sintering method and conventional solid-state reaction process, and the dependence of microstructure and energy storage properties of the ceramics on sintering approaches has been studied. The results reveal that not only the microstructure, but also the electrical properties of the PBLZST AFE ceramics are significantly improved by using the hot-press sintering method. Samples resulting from the hot-press sintering process have high breakdown strength of 180 kV/cm which results from the increase of density. Coupled with large polarization, the hotpressed AFE ceramics are shown to have a high recoverable energy density of 3.2 J/cm3. The recoverable energy density of the hot-pressed PBLZST AFE ceramics is 100{\%} greater than the conventional sintered specimens with recoverable energy density of 1.6 J/cm3.",
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High-energy storage performance of (Pb0.87Ba0.1la0.02)(Zr0.68Sn0.24Ti0.08)O3 antiferroelectric ceramics fabricated by the hot-press sintering method. / Zhang, Guangzu; Zhu, Dingyang; Zhang, Xiaoshan; Zhang, Ling; Yi, Jinqiao; Xie, Bing; Zeng, Yike; Li, Qi; Wang, Qing; Jiang, Shenglin.

In: Journal of the American Ceramic Society, Vol. 98, No. 4, 01.01.2015, p. 1175-1181.

Research output: Contribution to journalArticle

TY - JOUR

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AU - Zhang, Guangzu

AU - Zhu, Dingyang

AU - Zhang, Xiaoshan

AU - Zhang, Ling

AU - Yi, Jinqiao

AU - Xie, Bing

AU - Zeng, Yike

AU - Li, Qi

AU - Wang, Qing

AU - Jiang, Shenglin

PY - 2015/1/1

Y1 - 2015/1/1

N2 - (Pb0.87Ba0.1La0.02)(Zr0.68Sn0.24Ti0.08)O3 (PBLZST) antiferroelectric (AFE) ceramics have been prepared by hot-press sintering method and conventional solid-state reaction process, and the dependence of microstructure and energy storage properties of the ceramics on sintering approaches has been studied. The results reveal that not only the microstructure, but also the electrical properties of the PBLZST AFE ceramics are significantly improved by using the hot-press sintering method. Samples resulting from the hot-press sintering process have high breakdown strength of 180 kV/cm which results from the increase of density. Coupled with large polarization, the hotpressed AFE ceramics are shown to have a high recoverable energy density of 3.2 J/cm3. The recoverable energy density of the hot-pressed PBLZST AFE ceramics is 100% greater than the conventional sintered specimens with recoverable energy density of 1.6 J/cm3.

AB - (Pb0.87Ba0.1La0.02)(Zr0.68Sn0.24Ti0.08)O3 (PBLZST) antiferroelectric (AFE) ceramics have been prepared by hot-press sintering method and conventional solid-state reaction process, and the dependence of microstructure and energy storage properties of the ceramics on sintering approaches has been studied. The results reveal that not only the microstructure, but also the electrical properties of the PBLZST AFE ceramics are significantly improved by using the hot-press sintering method. Samples resulting from the hot-press sintering process have high breakdown strength of 180 kV/cm which results from the increase of density. Coupled with large polarization, the hotpressed AFE ceramics are shown to have a high recoverable energy density of 3.2 J/cm3. The recoverable energy density of the hot-pressed PBLZST AFE ceramics is 100% greater than the conventional sintered specimens with recoverable energy density of 1.6 J/cm3.

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