The results of vibrational echo correlation spectroscopy with full phase information were used to examine aspects of the hydrogen bond dynamics of methanol-OD in CCl4. By using extremely short pulses, it was possible to excite the entire very broad hydroxyl-stretching band including the 1-2 transition. Vibrational echo correlation spectroscopy combined with detailed calculations made it possible to explicate the population dynamics of hydrogen bond evolution with considerable clarity and detail.
All Science Journal Classification (ASJC) codes
- Physics and Astronomy(all)
- Physical and Theoretical Chemistry