Hydrogen Separation by Zeolite Membranes

Xiaochun Xu; Weishen Yang; Chunshan Song; Jie Liu; Liwu Lin

Hydrogen Separation by Zeolite Membranes

Xiaochun Xu, Weishen Yang, Chunshan Song, Jie Liu, Liwu Lin

Research output: Contribution to journal › Conference article › peer-review

Abstract

With the introduction of fuel cells for vehicular propulsion and power generation, hydrogen demand may increase significantly. The separation of hydrogen from its source gas mixtures is often the first step for the hydrogen applications. Thus, the synthesis and hydrogen separation properties of MFI and NaA zeolite membrane were studied. The NaA zeolite membrane showed a H₂ permeance of 2.86 × 10^-7 mole/sq m-sec-Pa. The H₂/N₂ and H₂/n-C₄H₁₀ permselectivity was 23.8 and 106, respectively, at 298 K. With the increase in permeation temperature, gas permeance increased. The H₂/N₂ and H₂n-C₄H₁₀ permselectivity gradually decreased with the increase in permeation temperature. Both MFI and NaA zeolite membrane showed a high H₂/n-C₄H₁₀ permselectivity.

Original language	English (US)
Pages (from-to)	284-285
Number of pages	2
Journal	ACS Division of Fuel Chemistry, Preprints
Volume	48
Issue number	1
State	Published - Mar 1 2003
Event	Proceedings of the 2003 SPE/EPA/DOE Exploration Production Environmental Conference - San Antonio, TX, United States Duration: Mar 10 2003 → Mar 12 2003

All Science Journal Classification (ASJC) codes

Energy(all)

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title = "Hydrogen Separation by Zeolite Membranes",

abstract = "With the introduction of fuel cells for vehicular propulsion and power generation, hydrogen demand may increase significantly. The separation of hydrogen from its source gas mixtures is often the first step for the hydrogen applications. Thus, the synthesis and hydrogen separation properties of MFI and NaA zeolite membrane were studied. The NaA zeolite membrane showed a H2 permeance of 2.86 × 10-7 mole/sq m-sec-Pa. The H2/N2 and H2/n-C4H10 permselectivity was 23.8 and 106, respectively, at 298 K. With the increase in permeation temperature, gas permeance increased. The H2/N2 and H2n-C4H10 permselectivity gradually decreased with the increase in permeation temperature. Both MFI and NaA zeolite membrane showed a high H2/n-C4H10 permselectivity.",

author = "Xiaochun Xu and Weishen Yang and Chunshan Song and Jie Liu and Liwu Lin",

year = "2003",

month = mar,

day = "1",

language = "English (US)",

volume = "48",

pages = "284--285",

journal = "Am Chem Soc Div Fuel Chem Prepr",

issn = "0569-3772",

number = "1",

note = "Proceedings of the 2003 SPE/EPA/DOE Exploration Production Environmental Conference ; Conference date: 10-03-2003 Through 12-03-2003",

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TY - JOUR

T1 - Hydrogen Separation by Zeolite Membranes

AU - Xu, Xiaochun

AU - Yang, Weishen

AU - Song, Chunshan

AU - Liu, Jie

AU - Lin, Liwu

PY - 2003/3/1

Y1 - 2003/3/1

N2 - With the introduction of fuel cells for vehicular propulsion and power generation, hydrogen demand may increase significantly. The separation of hydrogen from its source gas mixtures is often the first step for the hydrogen applications. Thus, the synthesis and hydrogen separation properties of MFI and NaA zeolite membrane were studied. The NaA zeolite membrane showed a H2 permeance of 2.86 × 10-7 mole/sq m-sec-Pa. The H2/N2 and H2/n-C4H10 permselectivity was 23.8 and 106, respectively, at 298 K. With the increase in permeation temperature, gas permeance increased. The H2/N2 and H2n-C4H10 permselectivity gradually decreased with the increase in permeation temperature. Both MFI and NaA zeolite membrane showed a high H2/n-C4H10 permselectivity.

AB - With the introduction of fuel cells for vehicular propulsion and power generation, hydrogen demand may increase significantly. The separation of hydrogen from its source gas mixtures is often the first step for the hydrogen applications. Thus, the synthesis and hydrogen separation properties of MFI and NaA zeolite membrane were studied. The NaA zeolite membrane showed a H2 permeance of 2.86 × 10-7 mole/sq m-sec-Pa. The H2/N2 and H2/n-C4H10 permselectivity was 23.8 and 106, respectively, at 298 K. With the increase in permeation temperature, gas permeance increased. The H2/N2 and H2n-C4H10 permselectivity gradually decreased with the increase in permeation temperature. Both MFI and NaA zeolite membrane showed a high H2/n-C4H10 permselectivity.

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M3 - Conference article

AN - SCOPUS:0345415715

VL - 48

SP - 284

EP - 285

JO - Am Chem Soc Div Fuel Chem Prepr

JF - Am Chem Soc Div Fuel Chem Prepr

SN - 0569-3772

IS - 1

T2 - Proceedings of the 2003 SPE/EPA/DOE Exploration Production Environmental Conference

Y2 - 10 March 2003 through 12 March 2003

ER -