Measurement of coherent polarons in the strongly coupled antiferromagnetically ordered iron-chalcogenide Fe1.02Te using angle-resolved photoemission spectroscopy

Z. K. Liu, R. H. He, D. H. Lu, M. Yi, Y. L. Chen, M. Hashimoto, R. G. Moore, S. K. Mo, E. A. Nowadnick, J. Hu, T. J. Liu, Z. Q. Mao, T. P. Devereaux, Z. Hussain, Z. X. Shen

Research output: Contribution to journalArticle

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Abstract

The nature of metallicity and the level of electronic correlations in the antiferromagnetically ordered parent compounds are two important open issues for the iron-based superconductivity. We perform a temperature-dependent angle-resolved photoemission spectroscopy study of Fe1.02Te, the parent compound for iron chalcogenide superconductors. Deep in the antiferromagnetic state, the spectra exhibit a "peak-dip-hump" line shape associated with two clearly separate branches of dispersion, characteristics of polarons seen in manganites and lightly doped cuprates. As temperature increases towards the Néel temperature (TN), we observe a decreasing renormalization of the peak dispersion and a counterintuitive sharpening of the hump linewidth, suggestive of an intimate connection between the weakening electron-phonon (e-ph) coupling and antiferromagnetism. Our finding points to the highly correlated nature of the Fe1.02Te ground state featured by strong interactions among the charge, spin, and lattice and a good metallicity plausibly contributed by the coherent polaron motion.

Original languageEnglish (US)
Article number037003
JournalPhysical Review Letters
Volume110
Issue number3
DOIs
StatePublished - Jan 18 2013

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polarons
photoelectric emission
iron
metallicity
spectroscopy
antiferromagnetism
cuprates
temperature
line shape
superconductivity
ground state
electronics
electrons

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy(all)

Cite this

Liu, Z. K. ; He, R. H. ; Lu, D. H. ; Yi, M. ; Chen, Y. L. ; Hashimoto, M. ; Moore, R. G. ; Mo, S. K. ; Nowadnick, E. A. ; Hu, J. ; Liu, T. J. ; Mao, Z. Q. ; Devereaux, T. P. ; Hussain, Z. ; Shen, Z. X. / Measurement of coherent polarons in the strongly coupled antiferromagnetically ordered iron-chalcogenide Fe1.02Te using angle-resolved photoemission spectroscopy. In: Physical Review Letters. 2013 ; Vol. 110, No. 3.
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abstract = "The nature of metallicity and the level of electronic correlations in the antiferromagnetically ordered parent compounds are two important open issues for the iron-based superconductivity. We perform a temperature-dependent angle-resolved photoemission spectroscopy study of Fe1.02Te, the parent compound for iron chalcogenide superconductors. Deep in the antiferromagnetic state, the spectra exhibit a {"}peak-dip-hump{"} line shape associated with two clearly separate branches of dispersion, characteristics of polarons seen in manganites and lightly doped cuprates. As temperature increases towards the N{\'e}el temperature (TN), we observe a decreasing renormalization of the peak dispersion and a counterintuitive sharpening of the hump linewidth, suggestive of an intimate connection between the weakening electron-phonon (e-ph) coupling and antiferromagnetism. Our finding points to the highly correlated nature of the Fe1.02Te ground state featured by strong interactions among the charge, spin, and lattice and a good metallicity plausibly contributed by the coherent polaron motion.",
author = "Liu, {Z. K.} and He, {R. H.} and Lu, {D. H.} and M. Yi and Chen, {Y. L.} and M. Hashimoto and Moore, {R. G.} and Mo, {S. K.} and Nowadnick, {E. A.} and J. Hu and Liu, {T. J.} and Mao, {Z. Q.} and Devereaux, {T. P.} and Z. Hussain and Shen, {Z. X.}",
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Liu, ZK, He, RH, Lu, DH, Yi, M, Chen, YL, Hashimoto, M, Moore, RG, Mo, SK, Nowadnick, EA, Hu, J, Liu, TJ, Mao, ZQ, Devereaux, TP, Hussain, Z & Shen, ZX 2013, 'Measurement of coherent polarons in the strongly coupled antiferromagnetically ordered iron-chalcogenide Fe1.02Te using angle-resolved photoemission spectroscopy', Physical Review Letters, vol. 110, no. 3, 037003. https://doi.org/10.1103/PhysRevLett.110.037003

Measurement of coherent polarons in the strongly coupled antiferromagnetically ordered iron-chalcogenide Fe1.02Te using angle-resolved photoemission spectroscopy. / Liu, Z. K.; He, R. H.; Lu, D. H.; Yi, M.; Chen, Y. L.; Hashimoto, M.; Moore, R. G.; Mo, S. K.; Nowadnick, E. A.; Hu, J.; Liu, T. J.; Mao, Z. Q.; Devereaux, T. P.; Hussain, Z.; Shen, Z. X.

In: Physical Review Letters, Vol. 110, No. 3, 037003, 18.01.2013.

Research output: Contribution to journalArticle

TY - JOUR

T1 - Measurement of coherent polarons in the strongly coupled antiferromagnetically ordered iron-chalcogenide Fe1.02Te using angle-resolved photoemission spectroscopy

AU - Liu, Z. K.

AU - He, R. H.

AU - Lu, D. H.

AU - Yi, M.

AU - Chen, Y. L.

AU - Hashimoto, M.

AU - Moore, R. G.

AU - Mo, S. K.

AU - Nowadnick, E. A.

AU - Hu, J.

AU - Liu, T. J.

AU - Mao, Z. Q.

AU - Devereaux, T. P.

AU - Hussain, Z.

AU - Shen, Z. X.

PY - 2013/1/18

Y1 - 2013/1/18

N2 - The nature of metallicity and the level of electronic correlations in the antiferromagnetically ordered parent compounds are two important open issues for the iron-based superconductivity. We perform a temperature-dependent angle-resolved photoemission spectroscopy study of Fe1.02Te, the parent compound for iron chalcogenide superconductors. Deep in the antiferromagnetic state, the spectra exhibit a "peak-dip-hump" line shape associated with two clearly separate branches of dispersion, characteristics of polarons seen in manganites and lightly doped cuprates. As temperature increases towards the Néel temperature (TN), we observe a decreasing renormalization of the peak dispersion and a counterintuitive sharpening of the hump linewidth, suggestive of an intimate connection between the weakening electron-phonon (e-ph) coupling and antiferromagnetism. Our finding points to the highly correlated nature of the Fe1.02Te ground state featured by strong interactions among the charge, spin, and lattice and a good metallicity plausibly contributed by the coherent polaron motion.

AB - The nature of metallicity and the level of electronic correlations in the antiferromagnetically ordered parent compounds are two important open issues for the iron-based superconductivity. We perform a temperature-dependent angle-resolved photoemission spectroscopy study of Fe1.02Te, the parent compound for iron chalcogenide superconductors. Deep in the antiferromagnetic state, the spectra exhibit a "peak-dip-hump" line shape associated with two clearly separate branches of dispersion, characteristics of polarons seen in manganites and lightly doped cuprates. As temperature increases towards the Néel temperature (TN), we observe a decreasing renormalization of the peak dispersion and a counterintuitive sharpening of the hump linewidth, suggestive of an intimate connection between the weakening electron-phonon (e-ph) coupling and antiferromagnetism. Our finding points to the highly correlated nature of the Fe1.02Te ground state featured by strong interactions among the charge, spin, and lattice and a good metallicity plausibly contributed by the coherent polaron motion.

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