NanoVelcro: Theory of Guided Folding in Atomically Thin Sheets with Regions of Complementary Doping

Research output: Contribution to journalArticle

3 Scopus citations

Abstract

Folding has been commonly observed in two-dimensional materials such as graphene and monolayer transition metal dichalcogenides. Although interlayer coupling stabilizes these folds, it provides no control over the placement of the fold, let alone the final folded shape. Lacking nanoscale "fingers" to externally guide folding, control requires interactions engineered into the sheets that guide them toward a desired final folded structure. Here we provide a theoretical framework for a general methodology toward this end: atomically thin 2D sheets are doped with patterns of complementary n-type and p-type regions whose preferential adhesion favors folding into desired shapes. The two-colorable theorem in flat-foldable origami ensures that arbitrary folding patterns are in principle accessible to this method. This complementary doping method can be combined with nanoscale crumpling (by, for example, passage of 2D sheets through holes) to obtain not only control over fold placements but also the ability to distinguish between degenerate folded states, thus attaining nontrivial shapes inaccessible to sequential folding.

Original languageEnglish (US)
Pages (from-to)6708-6714
Number of pages7
JournalNano letters
Volume17
Issue number11
DOIs
StatePublished - Nov 8 2017

All Science Journal Classification (ASJC) codes

  • Bioengineering
  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanical Engineering

Fingerprint Dive into the research topics of 'NanoVelcro: Theory of Guided Folding in Atomically Thin Sheets with Regions of Complementary Doping'. Together they form a unique fingerprint.

  • Cite this