Negative differential conductance & hot-carrier avalanching in monolayer WS2 FETs

G. He, J. Nathawat, C. P. Kwan, H. Ramamoorthy, R. Somphonsane, M. Zhao, K. Ghosh, U. Singisetti, N. Perea-López, C. Zhou, A. L. Elías, M. Terrones, Y. Gong, X. Zhang, R. Vajtai, P. M. Ajayan, D. K. Ferry, J. P. Bird

Research output: Contribution to journalArticle

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Abstract

The high field phenomena of inter-valley transfer and avalanching breakdown have long been exploited in devices based on conventional semiconductors. In this Article, we demonstrate the manifestation of these effects in atomically-thin WS2 field-effect transistors. The negative differential conductance exhibits all of the features familiar from discussions of this phenomenon in bulk semiconductors, including hysteresis in the transistor characteristics and increased noise that is indicative of travelling high-field domains. It is also found to be sensitive to thermal annealing, a result that we attribute to the influence of strain on the energy separation of the different valleys involved in hot-electron transfer. This idea is supported by the results of ensemble Monte Carlo simulations, which highlight the sensitivity of the negative differential conductance to the equilibrium populations of the different valleys. At high drain currents (>10 μA/μm) avalanching breakdown is also observed, and is attributed to trap-assisted inverse Auger scattering. This mechanism is not normally relevant in conventional semiconductors, but is possible in WS2 due to the narrow width of its energy bands. The various results presented here suggest that WS2 exhibits strong potential for use in hot-electron devices, including compact high-frequency sources and photonic detectors.

Original languageEnglish (US)
Article number11256
JournalScientific reports
Volume7
Issue number1
DOIs
StatePublished - Dec 1 2017

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Semiconductors
Electrons
Optics and Photonics
Equipment and Supplies
Noise
Hot Temperature
Population

All Science Journal Classification (ASJC) codes

  • General

Cite this

He, G., Nathawat, J., Kwan, C. P., Ramamoorthy, H., Somphonsane, R., Zhao, M., ... Bird, J. P. (2017). Negative differential conductance & hot-carrier avalanching in monolayer WS2 FETs. Scientific reports, 7(1), [11256]. https://doi.org/10.1038/s41598-017-11647-6
He, G. ; Nathawat, J. ; Kwan, C. P. ; Ramamoorthy, H. ; Somphonsane, R. ; Zhao, M. ; Ghosh, K. ; Singisetti, U. ; Perea-López, N. ; Zhou, C. ; Elías, A. L. ; Terrones, M. ; Gong, Y. ; Zhang, X. ; Vajtai, R. ; Ajayan, P. M. ; Ferry, D. K. ; Bird, J. P. / Negative differential conductance & hot-carrier avalanching in monolayer WS2 FETs. In: Scientific reports. 2017 ; Vol. 7, No. 1.
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abstract = "The high field phenomena of inter-valley transfer and avalanching breakdown have long been exploited in devices based on conventional semiconductors. In this Article, we demonstrate the manifestation of these effects in atomically-thin WS2 field-effect transistors. The negative differential conductance exhibits all of the features familiar from discussions of this phenomenon in bulk semiconductors, including hysteresis in the transistor characteristics and increased noise that is indicative of travelling high-field domains. It is also found to be sensitive to thermal annealing, a result that we attribute to the influence of strain on the energy separation of the different valleys involved in hot-electron transfer. This idea is supported by the results of ensemble Monte Carlo simulations, which highlight the sensitivity of the negative differential conductance to the equilibrium populations of the different valleys. At high drain currents (>10 μA/μm) avalanching breakdown is also observed, and is attributed to trap-assisted inverse Auger scattering. This mechanism is not normally relevant in conventional semiconductors, but is possible in WS2 due to the narrow width of its energy bands. The various results presented here suggest that WS2 exhibits strong potential for use in hot-electron devices, including compact high-frequency sources and photonic detectors.",
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He, G, Nathawat, J, Kwan, CP, Ramamoorthy, H, Somphonsane, R, Zhao, M, Ghosh, K, Singisetti, U, Perea-López, N, Zhou, C, Elías, AL, Terrones, M, Gong, Y, Zhang, X, Vajtai, R, Ajayan, PM, Ferry, DK & Bird, JP 2017, 'Negative differential conductance & hot-carrier avalanching in monolayer WS2 FETs', Scientific reports, vol. 7, no. 1, 11256. https://doi.org/10.1038/s41598-017-11647-6

Negative differential conductance & hot-carrier avalanching in monolayer WS2 FETs. / He, G.; Nathawat, J.; Kwan, C. P.; Ramamoorthy, H.; Somphonsane, R.; Zhao, M.; Ghosh, K.; Singisetti, U.; Perea-López, N.; Zhou, C.; Elías, A. L.; Terrones, M.; Gong, Y.; Zhang, X.; Vajtai, R.; Ajayan, P. M.; Ferry, D. K.; Bird, J. P.

In: Scientific reports, Vol. 7, No. 1, 11256, 01.12.2017.

Research output: Contribution to journalArticle

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AU - He, G.

AU - Nathawat, J.

AU - Kwan, C. P.

AU - Ramamoorthy, H.

AU - Somphonsane, R.

AU - Zhao, M.

AU - Ghosh, K.

AU - Singisetti, U.

AU - Perea-López, N.

AU - Zhou, C.

AU - Elías, A. L.

AU - Terrones, M.

AU - Gong, Y.

AU - Zhang, X.

AU - Vajtai, R.

AU - Ajayan, P. M.

AU - Ferry, D. K.

AU - Bird, J. P.

PY - 2017/12/1

Y1 - 2017/12/1

N2 - The high field phenomena of inter-valley transfer and avalanching breakdown have long been exploited in devices based on conventional semiconductors. In this Article, we demonstrate the manifestation of these effects in atomically-thin WS2 field-effect transistors. The negative differential conductance exhibits all of the features familiar from discussions of this phenomenon in bulk semiconductors, including hysteresis in the transistor characteristics and increased noise that is indicative of travelling high-field domains. It is also found to be sensitive to thermal annealing, a result that we attribute to the influence of strain on the energy separation of the different valleys involved in hot-electron transfer. This idea is supported by the results of ensemble Monte Carlo simulations, which highlight the sensitivity of the negative differential conductance to the equilibrium populations of the different valleys. At high drain currents (>10 μA/μm) avalanching breakdown is also observed, and is attributed to trap-assisted inverse Auger scattering. This mechanism is not normally relevant in conventional semiconductors, but is possible in WS2 due to the narrow width of its energy bands. The various results presented here suggest that WS2 exhibits strong potential for use in hot-electron devices, including compact high-frequency sources and photonic detectors.

AB - The high field phenomena of inter-valley transfer and avalanching breakdown have long been exploited in devices based on conventional semiconductors. In this Article, we demonstrate the manifestation of these effects in atomically-thin WS2 field-effect transistors. The negative differential conductance exhibits all of the features familiar from discussions of this phenomenon in bulk semiconductors, including hysteresis in the transistor characteristics and increased noise that is indicative of travelling high-field domains. It is also found to be sensitive to thermal annealing, a result that we attribute to the influence of strain on the energy separation of the different valleys involved in hot-electron transfer. This idea is supported by the results of ensemble Monte Carlo simulations, which highlight the sensitivity of the negative differential conductance to the equilibrium populations of the different valleys. At high drain currents (>10 μA/μm) avalanching breakdown is also observed, and is attributed to trap-assisted inverse Auger scattering. This mechanism is not normally relevant in conventional semiconductors, but is possible in WS2 due to the narrow width of its energy bands. The various results presented here suggest that WS2 exhibits strong potential for use in hot-electron devices, including compact high-frequency sources and photonic detectors.

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He G, Nathawat J, Kwan CP, Ramamoorthy H, Somphonsane R, Zhao M et al. Negative differential conductance & hot-carrier avalanching in monolayer WS2 FETs. Scientific reports. 2017 Dec 1;7(1). 11256. https://doi.org/10.1038/s41598-017-11647-6