@article{a8835f4b5080460aa8c9a83eebb1cefe,
title = "Oxygen octahedral tilt ordering in (Na1/2Bi1/2)TiO3 ferroelectric thin films",
abstract = "Oxygen octahedra tilt (OOT) transition is the most common type of distortion in inorganic ABO3 compounds with a perovskite crystal structure. The importance of OOT transitions is underlined by accompanying changes in the B-O and A-O bonding environments, which consequently affects the electronic states and hence influences electrical, magnetic, and superconducting properties of many perovskite compounds. In recent years, controlled manipulation of the OOT order in perovskite thin film ferroelectrics has been attempted through heteroepitaxial strain engineering. The current study demonstrates an alternative approach whereby OOT ordering in a 200 nm thick polycrystalline thin film of (Na1/2Bi1/2)TiO3 (NBT) Pb-free ferroelectric is induced by applying electric-field along the 111 octahedral tilt axis, which is furthermore enabled by a strong (111) crystallographic texture normal to the film surface. In situ x-ray diffraction reveals that electric-field-induced OOT ordering proceeds through nucleation and rapid growth of domains with ordered a-a-a- tilting, followed by an increase in the tilt angle within the ordered domains.",
author = "A. Pramanick and Paterson, {A. R.} and L. Denis and W. Abbas and G. Niu and W. Ren and J. Zhao and L. Dai and O. Borkiewicz and Y. Ren and D. Ho and S. Trolier-Mckinstry and Jones, {J. L.}",
note = "Funding Information: A.P. and W.A. gratefully acknowledge funding support from CityU (Projects Nos. 7200514 and 9610377). G.N., W.R., J.Z., and L.D. acknowledge support from the National Natural Science Foundation of China (No. 51602247), Natural Science Fundamental Research Project of Shaanxi Province of China (No. 2017JQ6003), the Fundamental Research Funds for the Central Universities and the Natural Sciences and Engineering Research Council, and Selected Foundation for Science and Technology Activities of Returned Chinese Scholars. S.T.M. and L.D. gratefully acknowledge support from the U.S. National Science Foundation (No. DMR-1410907). A.R.P. and J.L.J. gratefully acknowledge support from the U.S. National Science Foundation (No. DMR-1409399). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. Technical assistance from Richard A. Spence at Advanced Photon Source is gratefully acknowledged.",
year = "2020",
month = jan,
day = "13",
doi = "10.1063/1.5127212",
language = "English (US)",
volume = "116",
journal = "Applied Physics Letters",
issn = "0003-6951",
publisher = "American Institute of Physics Publising LLC",
number = "2",
}