Polaritonic Hybrid-Epsilon-near-Zero Modes: Beating the Plasmonic Confinement vs Propagation-Length Trade-Off with Doped Cadmium Oxide Bilayers

Evan L. Runnerstrom, Kyle P. Kelley, Thomas G. Folland, J. Ryan Nolen, Nader Engheta, Joshua D. Caldwell, Jon-Paul Maria

Research output: Contribution to journalArticle

6 Citations (Scopus)

Abstract

Polaritonic materials that support epsilon-near-zero (ENZ) modes offer the opportunity to design light-matter interactions at the nanoscale through extreme subwavelength light confinement, producing phenomena like resonant perfect absorption. However, the utility of ENZ modes in nanophotonic applications has been limited by a flat spectral dispersion, which leads to small group velocities and extremely short propagation lengths. Here, we overcome this constraint by hybridizing ENZ and surface plasmon polariton (SPP) modes in doped cadmium oxide epitaxial bilayers. This results in strongly coupled hybrid modes that are characterized by an anticrossing in the polariton dispersion and a large spectral splitting on the order of 1/3 of the mode frequency. These hybrid modes simultaneously achieve modal propagation and ENZ mode-like interior field confinement, adding propagation character to ENZ mode properties. We subsequently tune the resonant frequencies, dispersion, and coupling of these polaritonic-hybrid-epsilon-near-zero (PH-ENZ) modes by tailoring the modal oscillator strength and the ENZ-SPP spectral overlap. PH-ENZ modes ultimately leverage the most desirable characteristics of both ENZ and SPP modes, allowing us to overcome the canonical plasmonic trade-off between confinement and propagation length.

Original languageEnglish (US)
Pages (from-to)948-957
Number of pages10
JournalNano letters
Volume19
Issue number2
DOIs
StatePublished - Feb 13 2019

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Cadmium
cadmium
Oxides
oxides
propagation
Nanophotonics
polaritons
Laser modes
Natural frequencies
cadmium oxide
propagation modes
group velocity
oscillator strengths
resonant frequencies

All Science Journal Classification (ASJC) codes

  • Bioengineering
  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanical Engineering

Cite this

Runnerstrom, Evan L. ; Kelley, Kyle P. ; Folland, Thomas G. ; Nolen, J. Ryan ; Engheta, Nader ; Caldwell, Joshua D. ; Maria, Jon-Paul. / Polaritonic Hybrid-Epsilon-near-Zero Modes : Beating the Plasmonic Confinement vs Propagation-Length Trade-Off with Doped Cadmium Oxide Bilayers. In: Nano letters. 2019 ; Vol. 19, No. 2. pp. 948-957.
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abstract = "Polaritonic materials that support epsilon-near-zero (ENZ) modes offer the opportunity to design light-matter interactions at the nanoscale through extreme subwavelength light confinement, producing phenomena like resonant perfect absorption. However, the utility of ENZ modes in nanophotonic applications has been limited by a flat spectral dispersion, which leads to small group velocities and extremely short propagation lengths. Here, we overcome this constraint by hybridizing ENZ and surface plasmon polariton (SPP) modes in doped cadmium oxide epitaxial bilayers. This results in strongly coupled hybrid modes that are characterized by an anticrossing in the polariton dispersion and a large spectral splitting on the order of 1/3 of the mode frequency. These hybrid modes simultaneously achieve modal propagation and ENZ mode-like interior field confinement, adding propagation character to ENZ mode properties. We subsequently tune the resonant frequencies, dispersion, and coupling of these polaritonic-hybrid-epsilon-near-zero (PH-ENZ) modes by tailoring the modal oscillator strength and the ENZ-SPP spectral overlap. PH-ENZ modes ultimately leverage the most desirable characteristics of both ENZ and SPP modes, allowing us to overcome the canonical plasmonic trade-off between confinement and propagation length.",
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Polaritonic Hybrid-Epsilon-near-Zero Modes : Beating the Plasmonic Confinement vs Propagation-Length Trade-Off with Doped Cadmium Oxide Bilayers. / Runnerstrom, Evan L.; Kelley, Kyle P.; Folland, Thomas G.; Nolen, J. Ryan; Engheta, Nader; Caldwell, Joshua D.; Maria, Jon-Paul.

In: Nano letters, Vol. 19, No. 2, 13.02.2019, p. 948-957.

Research output: Contribution to journalArticle

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T2 - Beating the Plasmonic Confinement vs Propagation-Length Trade-Off with Doped Cadmium Oxide Bilayers

AU - Runnerstrom, Evan L.

AU - Kelley, Kyle P.

AU - Folland, Thomas G.

AU - Nolen, J. Ryan

AU - Engheta, Nader

AU - Caldwell, Joshua D.

AU - Maria, Jon-Paul

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