Two-photon-pumped lasing from colloidal nanocrystal quantum dots

Chunfeng Zhang, Fan Zhang, Ting Zhu, An Cheng, Jian Xu, Qi Zhang, Suzanne E. Mohney, Ron H. Henderson, Y. Andrew Wang

Research output: Contribution to journalArticlepeer-review

41 Scopus citations

Abstract

Upconverted lasing in the nonlinear, two-photon absorption regime has been demonstrated, for the first time to the best of our knowledge in colloidal nanocrystal quantum dots (NQDs). Upon pulse excitation at sub-bandgap photon energies the radiative recombination of excitons in close-packed CdSe/CdS/ZnS core-shell NQDs was found to be sufficiently fast to compete with the intrinsic nonradiative Auger recombination, as confirmed by the presence of a fast decay (∼7 ps) in the time-resolved photoluminescence.

Original languageEnglish (US)
Pages (from-to)2437-2439
Number of pages3
JournalOptics Letters
Volume33
Issue number21
DOIs
StatePublished - Nov 1 2008

All Science Journal Classification (ASJC) codes

  • Atomic and Molecular Physics, and Optics

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