Unveiling non-equilibrium metallurgical phases in dissimilar Al-Cu joints processed by vaporizing foil actuator welding

Kaifeng Wang, Shun Li Shang, Yuxiang Wang, Anupam Vivek, Glenn Daehn, Zi Kui Liu, Jingjing Li

Research output: Contribution to journalArticle

Abstract

An integrated experimental and computational approach has been adopted to investigate the formation mechanism of intermetallic compounds (IMCs) in dissimilar Al-Cu joints processed by vaporizing foil actuator welding (VFAW). Aiming to understand the formation of IMCs and their transition, the present work employed first-principles calculations of thermodynamic properties as a function of temperature and pressure together with diffusivities of Al and Cu from the literature. Agreeing with experimental observations, the predicted IMC formation sequence in the low-energy welding region is as follows. θ-Al2Cu forms first due to the fast diffusivity of Cu in the Al-matrix. θ-Al2Cu then transforms to η2-AlCu because of the fast diffusivities of Al/Cu in θ-Al2Cu. In the high-energy welding region, the stable γ1-Al4Cu9 and the metastable θ’’-Al3Cu are also formed in addition to the aforementioned θ-Al2Cu and η2-AlCu. η2-AlCu and considerable γ1-Al4Cu9 are the major phases in the high-energy welding region. The present approach, combining experiments and calculations, is proven to be a practical way to understand non-equilibrium metallurgical processes, as demonstrated through the study of VFAW Al-Cu joints.

Original languageEnglish (US)
Article number108306
JournalMaterials and Design
Volume186
DOIs
StatePublished - Jan 15 2020

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Vaporization
Metal foil
Welding
Actuators
Intermetallics
Thermodynamic properties
Experiments
Temperature

All Science Journal Classification (ASJC) codes

  • Materials Science(all)
  • Mechanics of Materials
  • Mechanical Engineering

Cite this

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title = "Unveiling non-equilibrium metallurgical phases in dissimilar Al-Cu joints processed by vaporizing foil actuator welding",
abstract = "An integrated experimental and computational approach has been adopted to investigate the formation mechanism of intermetallic compounds (IMCs) in dissimilar Al-Cu joints processed by vaporizing foil actuator welding (VFAW). Aiming to understand the formation of IMCs and their transition, the present work employed first-principles calculations of thermodynamic properties as a function of temperature and pressure together with diffusivities of Al and Cu from the literature. Agreeing with experimental observations, the predicted IMC formation sequence in the low-energy welding region is as follows. θ-Al2Cu forms first due to the fast diffusivity of Cu in the Al-matrix. θ-Al2Cu then transforms to η2-AlCu because of the fast diffusivities of Al/Cu in θ-Al2Cu. In the high-energy welding region, the stable γ1-Al4Cu9 and the metastable θ’’-Al3Cu are also formed in addition to the aforementioned θ-Al2Cu and η2-AlCu. η2-AlCu and considerable γ1-Al4Cu9 are the major phases in the high-energy welding region. The present approach, combining experiments and calculations, is proven to be a practical way to understand non-equilibrium metallurgical processes, as demonstrated through the study of VFAW Al-Cu joints.",
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Unveiling non-equilibrium metallurgical phases in dissimilar Al-Cu joints processed by vaporizing foil actuator welding. / Wang, Kaifeng; Shang, Shun Li; Wang, Yuxiang; Vivek, Anupam; Daehn, Glenn; Liu, Zi Kui; Li, Jingjing.

In: Materials and Design, Vol. 186, 108306, 15.01.2020.

Research output: Contribution to journalArticle

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AU - Shang, Shun Li

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AU - Vivek, Anupam

AU - Daehn, Glenn

AU - Liu, Zi Kui

AU - Li, Jingjing

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